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I agree that it's hard to predict what will provide outstanding value in the long-term. Looking at modern coinage, I doubt seriously that any one item will show the kind of increase that we've seen on older series like the Morgans.
If I had to guess, I'd bet my money on Modern Commemoratives, especially the gold issues and our only gold/platinum issue to-date. Just my 100 year opinion.
On non-modern, I'd say that everything in great condition will appreciate significantly. Great condition is series oriented. For example Large Cents and Half Cents in XF look great and are certainly hard to find.
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